真空膜蒸馏和膜吸收及其集成工艺处理高氨氮废水

段明星, 王建兵, 王军, 纪仲光. 真空膜蒸馏和膜吸收及其集成工艺处理高氨氮废水[J]. 环境工程学报, 2015, 9(2): 659-664. doi: 10.12030/j.cjee.20150225
引用本文: 段明星, 王建兵, 王军, 纪仲光. 真空膜蒸馏和膜吸收及其集成工艺处理高氨氮废水[J]. 环境工程学报, 2015, 9(2): 659-664. doi: 10.12030/j.cjee.20150225
Duan Mingxing, Wang Jianbing, Wang Jun, Ji Zhongguang. Vacuum membrane distillation and membrane absorption and integrated process for ammonia removal from wastewater[J]. Chinese Journal of Environmental Engineering, 2015, 9(2): 659-664. doi: 10.12030/j.cjee.20150225
Citation: Duan Mingxing, Wang Jianbing, Wang Jun, Ji Zhongguang. Vacuum membrane distillation and membrane absorption and integrated process for ammonia removal from wastewater[J]. Chinese Journal of Environmental Engineering, 2015, 9(2): 659-664. doi: 10.12030/j.cjee.20150225

真空膜蒸馏和膜吸收及其集成工艺处理高氨氮废水

  • 基金项目:

    国家自然科学基金资助项目(51378491)

    国家"水体污染控制与治理"科技重大专项(2012ZX07202006-003-2)

  • 中图分类号: TQ028.8

Vacuum membrane distillation and membrane absorption and integrated process for ammonia removal from wastewater

  • Fund Project:
  • 摘要: 采用PP中空纤维膜组件,对VMD(真空膜蒸馏)和MA(膜吸收)脱氨过程进行了研究。考察了料液pH值(9.0~11.0)、料液进口温度(20~50℃)对脱氨效率的影响。研究结果表明,VMD和MA脱除率分别达85%和99%以上。料液pH和料液进口温度对VMD脱氨效果的影响较大,提高料液pH和进口温度可以明显提高VMD的脱氨效率;料液pH对MA的脱氨效率影响较为显著。对2种膜工艺进行了技术集成,利用该集成工艺可达到99.96%以上的氨去除率,出水可达标排放,并且可以有效防止硫酸铵的二次污染。
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  • [1] 应德煌.氨氮废水治理方案的选择.福建化工,2003,(2):50-54 Ying D.H. Selection of treatment of Ammonia wastewater. Fujian Chemical, 2003, (2):50-54(in Chinese)
    [2] Cooney Emma L., Booker Nicholas A., Shallcross David C. Ammonia removal from waste water using natural Australian zeolite. I. Characterization of the zeolite. Separation Science and Technology, 1999, 34 (12):2307-2327
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    [4] Carrera J., Baeca J.A., Vicent T., et al. Biological nitrogen removal of high-strength ammonium industrial wastewater with two-sludge system. Water Research, 2003, 37(17): 4211-4221
    [5] 袁捷,杨宁,周艳军.吹脱法处理高浓度氨氮废水的研究.化学工业与工程技术,2009,30(4):55-57 Yuan J., Yang N., Zhou Y.J. Research on striping treatment of high concentrated ammonia nitrogen wastewater. Journal of Chemical Industry & Engineering,2009,30(4):55-57(in Chinese)
    [6] Jeffrey W.A. Charrois, Steve E.,et al. Breakpoint chlorination and free-chlorine contact time: Implications for drinking water N-nitrosodimethylamine concentrations. Water Research,2007,41(3): 674-682
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    [8] Huang C.M., Lou J.C., Lin C.H. Removal of ammonia solutions used in catalytic wet oxidation processes. Chemosphere, 2003, 52(6):989-995
    [9] Mandowara A., Prashant K., Bhattacharya. Simulation studies of ammonia removal from water in a membrane contactor under liquid-liquid extraction mode. Journal of Environmental Management, 2011, 92(1):121-130
    [10] Mondor M., Masse L., Ippersiel D.,et al. Use of electrodialysis and reverse osmosis for the recovery and concentration of ammonia from swine manure. Bioresource Technology, 2008, 99(15):7363-7368
    [11] Walker M., Iyer K., Heaven S., et al. Ammonia removal in anaerobic digestion by biogas stripping: An evaluation of process alternatives using a first order rate model based on experimental fimmonia Chemical Engineering Journal, 2011, 178(24):138-145
    [12] Garrido J.M., Guerrero L., Mendez R., et al. Nitification ofwaste waters from fish-meal factories.Water SA, 1998, 24(3):245-249
    [13] 黄伟.減压膜蒸馏法处理石煤提钒废水研究.武汉:武汉理工大学硕士学位论文,2012 Huang W. Vacuum membrane distillation treatment of wastewater produced in vanadium extraction from stone coal.Wuhan:Master Dissertation of Wuhan University of Technology, 2012 (in Chinese)
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  • 收稿日期:  2014-01-15
  • 刊出日期:  2015-02-07
段明星, 王建兵, 王军, 纪仲光. 真空膜蒸馏和膜吸收及其集成工艺处理高氨氮废水[J]. 环境工程学报, 2015, 9(2): 659-664. doi: 10.12030/j.cjee.20150225
引用本文: 段明星, 王建兵, 王军, 纪仲光. 真空膜蒸馏和膜吸收及其集成工艺处理高氨氮废水[J]. 环境工程学报, 2015, 9(2): 659-664. doi: 10.12030/j.cjee.20150225
Duan Mingxing, Wang Jianbing, Wang Jun, Ji Zhongguang. Vacuum membrane distillation and membrane absorption and integrated process for ammonia removal from wastewater[J]. Chinese Journal of Environmental Engineering, 2015, 9(2): 659-664. doi: 10.12030/j.cjee.20150225
Citation: Duan Mingxing, Wang Jianbing, Wang Jun, Ji Zhongguang. Vacuum membrane distillation and membrane absorption and integrated process for ammonia removal from wastewater[J]. Chinese Journal of Environmental Engineering, 2015, 9(2): 659-664. doi: 10.12030/j.cjee.20150225

真空膜蒸馏和膜吸收及其集成工艺处理高氨氮废水

  • 1.  中国矿业大学(北京)化学与环境工程学院, 北京 100083
  • 2.  中国科学院生态环境研究中心环境水质学国家重点实验室, 北京 100085
基金项目:

国家自然科学基金资助项目(51378491)

国家"水体污染控制与治理"科技重大专项(2012ZX07202006-003-2)

摘要: 采用PP中空纤维膜组件,对VMD(真空膜蒸馏)和MA(膜吸收)脱氨过程进行了研究。考察了料液pH值(9.0~11.0)、料液进口温度(20~50℃)对脱氨效率的影响。研究结果表明,VMD和MA脱除率分别达85%和99%以上。料液pH和料液进口温度对VMD脱氨效果的影响较大,提高料液pH和进口温度可以明显提高VMD的脱氨效率;料液pH对MA的脱氨效率影响较为显著。对2种膜工艺进行了技术集成,利用该集成工艺可达到99.96%以上的氨去除率,出水可达标排放,并且可以有效防止硫酸铵的二次污染。

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